Terahertz on David A. Reiss

Theory of ac magnetoelectric transport in normal-metal - magnetic-insulator heterostructures

Fri, 23 Aug 2024 00:00:00 +0000

(Note that cited here as the arXiv v1 preprint. The content was later reorganized (after disagreements about this I decided to be not included in the list of authors anymore) and published as Phys. Rev. B 113, 014419 (2026).) Electron-magnon coupling at the interface between a normal metal and a magnetically ordered insulator modifies the electrical conductivity of the normal metal, an effect known as spin-Hall magnetoresistance. It can also facilitate magnon-mediated current drag, the nonlocal electric current response of two normal metal layers separated by a magnetic insulator. In this article, we present a theory of these two spintronic effects and their nonlinear counterparts for time-dependent applied electric fields $E(\omega)$, with driving frequencies $\omega$ up to the THz regime. We compare various mechanisms leading to a quadratic-in-$E$ response - Joule heating, spin-torque diode effect, and magnonic unidirectional spin-Hall magnetoresistance - and show how these can be disentangled by their characteristic dependences on $\omega$ and the magnetization direction.

Ultrafast demagnetization of iron induced by optical versus terahertz pulses

Thu, 03 Jun 2021 00:00:00 +0000

We study ultrafast magnetization quenching of ferromagnetic iron following excitation by an optical vs a terahertz pump pulse. While the optical pump (photon energy of 3.1 eV) induces a strongly nonthermal electron distribution, terahertz excitation (~4 meV) results in a quasi-thermal perturbation of the electron population. The pump-induced spin and electron dynamics are interrogated by the magneto-optic Kerr effect (MOKE). A deconvolution procedure allows us to push the time resolution down to 130 fs, even though the driving terahertz pulse is more than 0.5 ps long. Remarkably, the MOKE signals exhibit an almost identical time evolution for both optical and terahertz pump pulses, despite the three orders of magnitude different number of excited electrons. We are able to quantitatively explain our results using a model based on quasi-elastic spin-flip scattering. It shows that in the small-perturbation limit, the rate of demagnetization of a metallic ferromagnet is proportional to the excess energy of the electrons, independent of the precise shape of their distribution. Our results reveal that the dynamics of ultrafast demagnetization and of the closely related terahertz spin transport do not depend on the pump photon energy.

Theory of spin-Hall magnetoresistance in the ac terahertz regime

Tue, 13 Apr 2021 00:00:00 +0000

In bilayers consisting of a normal metal (N) with spin-orbit coupling and a ferromagnet (F), the combination of the spin-Hall effect, the spin-transfer torque, and the inverse spin-Hall effect gives a small correction to the in-plane conductivity of N, which is referred to as spin-Hall magnetoresistance (SMR). We here present a theory of the SMR and the associated off-diagonal conductivity corrections for frequencies up to the terahertz regime. We show that the SMR signal has pronounced singularities at the spin-wave frequencies of F, which identifies it as a potential tool for all-electric spectroscopy of magnon modes. A systematic change of the magnitude of the SMR at lower frequencies is associated with the onset of a longitudinal magnonic contribution to spin transport across the F-N interface.

Laser-induced terahertz spin transport in magnetic nanostructures arises from the same force as ultrafast demagnetization

Mon, 22 Mar 2021 00:00:00 +0000

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably measure both processes in one setup. We find that the rate of UDM of a single ferromagnetic metal film F has the same time evolution as the flux of TST from F into an adjacent normal-metal layer N. This remarkable agreement shows that UDM and TST are driven by the same force, which is fully determined by the state of the ferromagnet. An analytical model consistently and quantitatively explains our observations. It reveals that both UDM in F and TST in the F|N stack arise from a generalized spin voltage, which is defined for arbitrary, nonthermal electron distributions. We also conclude that contributions due to a possible temperature difference between F and N are minor and that the spin-current amplitude can, in principle, be increased by one order of magnitude. In general, our findings allow one to apply the vast knowledge of UDM to TST, thereby opening up new pathways toward large-amplitude terahertz spin currents and, thus, energy-efficient ultrafast spintronic devices.